Americium incorporation into studtite: a theoretical and experimental study

Journal Article
Dalton Transactions, vol. 48, iss. 34, pp. 13057-13063, 2019
Authors
Saptarshi Biswas, Samuel J. Edwards, Zheming Wang, Hang Si, Luis León Vintró, Brendan Twamley, Piotr M. Kowalski, Robert J. Baker
Abstract

Reactions of [AmO2]+ with [UO22-O2)(H2O)2]·2H2O have been examined and the Am is reduced to Am(iii). Leaching experiments show that Am(iii) can be easily removed and a computational study sheds light on the mechanism and incorporation energies.

English